The use of stable lead 206207 isotope ratios and elemental composition to discriminate the origins of lead in aerosols at a rural site in eastern Canada

W.T Sturges , Barrie L.A
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引用次数: 89

Abstract

Observations of lead 206207 ratios and trace element concentrations in atmospheric aerosols at a rural location in Ontario, Canada confirm results of a previous study of urban aerosols that showed there are significant differences in the isotopic composition of lead from Canadian autos, Canadian smelters and eastern American sources. Lead measurements in fall 1984 and spring 1986 were apportioned to the respective sources as follows: for 1984 (55, 2, 43%) and for 1986 (69, 7, 24%). Lead isotopic and meteorological information point to In as the best elemental tracer of emissions from selected northern Canadian smelters.

使用稳定的铅206207同位素比率和元素组成来区分加拿大东部农村地区气溶胶中铅的来源
对加拿大安大略省农村地区大气气溶胶中铅206207比率和微量元素浓度的观察证实了先前对城市气溶胶的研究结果,即来自加拿大汽车、加拿大冶炼厂和美国东部来源的铅的同位素组成存在显著差异。1984年秋季和1986年春季的铅测量值被分配到各自的来源如下:1984年(55,2,43%)和1986年(69,7,24%)。铅同位素和气象资料指出,铅是加拿大北部某些冶炼厂排放的最佳元素示踪剂。
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