Solution-Processed Titanium Dioxide Ion-Gated Transistors and Their Application for pH Sensing

IF 1.9 Q3 ENGINEERING, ELECTRICAL & ELECTRONIC
Arunprabaharan Subramanian, Mona Azimi, Cheng Yee Leong, S. Lee, C. Santato, F. Cicoira
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引用次数: 1

Abstract

Titanium dioxide (TiO2) is an abundant metal oxide, widely used in food industry, cosmetics, medicine, water treatment and electronic devices. TiO2 is of interest for next-generation indium-free thin-film transistors and ion-gated transistors due to its tunable optoelectronic properties, ambient stability, and solution processability. In this work, we fabricated TiO2 films using a wet chemical approach and demonstrated their transistor behavior with room temperature ionic liquids and aqueous electrolytes. In addition, we demonstrated the pH sensing behavior of the TiO2 IGTs with a sensitivity of ∼48 mV/pH. Furthermore, we demonstrated a low temperature (120°C), solution processed TiO2-based IGTs on flexible polyethylene terephthalate (PET) substrates, which were stable under moderate tensile bending.
溶液处理二氧化钛离子门控晶体管及其在pH传感中的应用
二氧化钛(TiO2)是一种丰富的金属氧化物,广泛应用于食品工业、化妆品、医药、水处理和电子设备。TiO2由于其可调的光电特性、环境稳定性和溶液可加工性,在下一代无铟薄膜晶体管和离子门控晶体管中备受关注。在这项工作中,我们使用湿化学方法制备了TiO2薄膜,并展示了它们在室温离子液体和水性电解质中的晶体管行为。此外,我们还展示了TiO2 IGT的pH传感行为,其灵敏度为~48mV/pH。此外,我们在柔性聚对苯二甲酸乙二醇酯(PET)基底上展示了一种低温(120°C)溶液处理的TiO2基IGT,其在中等拉伸弯曲下是稳定的。
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