Fabrication of binary NiSe2–ZnS nanocomposites for high-performance supercapacitors with enhanced energy storage

IF 6.3 2区 材料科学 Q2 CHEMISTRY, PHYSICAL
Muhammad Sanaullah Shah, Zhang Zhenyu, Sohail Ahmad, Wang Shuiying, Hou Hongying, Zuo Xiaoqing, Muhammad Zia Ullah Shah
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Abstract

The development of supercapacitor technology has advanced significantly because of the high need for efficient and sustainable energy storage solutions. This study investigates the synthesis and electrochemical performance of NiSe2-ZnS nanocomposites as promising electrode materials for high-performance supercapacitor. The NiSe2-ZnS nanocomposites were synthesized via simple chemical method, and characterized. The results showed that the NiSe2-ZnS composite have outstanding electrochemical behaviors, combining the superior chemical stability and thermal durability of NiSe2 with the remarkable electrical conductivity of ZnS. The NiSe2-ZnS hybrid electrode demonstrated remarkable electrochemical behavior, delivering a specific capacitance of 810 F g-1 in a three-electrode system and 87.3 F g-1 when evaluated in a two-electrode configuration. It also demonstrated a notable energy density (ED) of 27.2 Wh/kg and a high power density (PD) of 3744.7 W/kg. Notably, the electrode retained 96.7% of its original capacitance even after 5000 continuous charge-discharge cycles conducted under a current load of 15 A g-1, demonstrating excellent cycling durability. This research shows that NiSe2-ZnS nanocomposites is a good-performance, low-cost, and sustainable material for next-generation supercapacitors.

Abstract Image

高性能储能超级电容器用NiSe2-ZnS二元纳米复合材料的制备
由于对高效和可持续的能源存储解决方案的高度需求,超级电容器技术的发展取得了显著进展。研究了NiSe2-ZnS纳米复合材料的合成及其电化学性能,该材料有望成为高性能超级电容器的电极材料。采用简单化学方法合成了NiSe2-ZnS纳米复合材料,并对其进行了表征。结果表明:NiSe2-ZnS复合材料具有优异的电化学性能,NiSe2优异的化学稳定性和热耐久性与ZnS优异的导电性相结合。NiSe2-ZnS混合电极表现出卓越的电化学行为,在三电极系统中提供810 F -1的比电容,在两电极配置中评估时提供87.3 F -1。其能量密度(ED)为27.2 Wh/kg,功率密度(PD)为3744.7 W/kg。值得注意的是,即使在15 a g-1的电流负载下进行5000次连续充放电循环后,电极仍保持了96.7%的原始电容,表现出优异的循环耐久性。研究表明,NiSe2-ZnS纳米复合材料是一种性能优良、成本低、可持续发展的下一代超级电容器材料。
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来源期刊
Surfaces and Interfaces
Surfaces and Interfaces Chemistry-General Chemistry
CiteScore
8.50
自引率
6.50%
发文量
753
审稿时长
35 days
期刊介绍: The aim of the journal is to provide a respectful outlet for ''sound science'' papers in all research areas on surfaces and interfaces. We define sound science papers as papers that describe new and well-executed research, but that do not necessarily provide brand new insights or are merely a description of research results. Surfaces and Interfaces publishes research papers in all fields of surface science which may not always find the right home on first submission to our Elsevier sister journals (Applied Surface, Surface and Coatings Technology, Thin Solid Films)
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