Mingyi Jiang, Zengcheng Yu, Linhan Yang, Prof. Fei Wang, Prof. Weidi Cao, Prof. Xiaohua Liu, Prof. Xiaoming Feng
{"title":"Frontispiz: Reductant-Free Enantioselective Aza-Reformatsky Reaction Enabled by Synergistic Visible Light Photocatalysis and Lewis Acid Catalysis","authors":"Mingyi Jiang, Zengcheng Yu, Linhan Yang, Prof. Fei Wang, Prof. Weidi Cao, Prof. Xiaohua Liu, Prof. Xiaoming Feng","doi":"10.1002/ange.202581762","DOIUrl":null,"url":null,"abstract":"<p>The visible-light and chiral-Lewis-acid synergistically catalyzed reductant-free asymmetric aza-Reformatsky reaction is described by Xiaoming Feng and co-workers in their Communication (e202500756). Control experiments revealed a direct SET process between excited state imine and α-iodo difluoromethyl carbonyl compound which prevents the use of reductant.\n <figure>\n <div><picture>\n <source></source></picture><p></p>\n </div>\n </figure>\n </p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 17","pages":""},"PeriodicalIF":0.0000,"publicationDate":"2025-04-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202581762","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Angewandte Chemie","FirstCategoryId":"1085","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/ange.202581762","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0
Abstract
The visible-light and chiral-Lewis-acid synergistically catalyzed reductant-free asymmetric aza-Reformatsky reaction is described by Xiaoming Feng and co-workers in their Communication (e202500756). Control experiments revealed a direct SET process between excited state imine and α-iodo difluoromethyl carbonyl compound which prevents the use of reductant.
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