{"title":"Highly Efficient Spin-Orbit Torque Switching in a Topological Insulator/Chromium Telluride Heterostructure with Opposite Berry Curvature","authors":"Kewen Zhang, Yuhang Wu, Jingyan Song, Yitian Guo, Xiaolun Cai, Long Cheng, Dongxing Zheng, Aitian Chen, Peng Li, Xixiang Zhang","doi":"10.1002/aelm.202400820","DOIUrl":null,"url":null,"abstract":"Energy-efficient magnetization switching by current-induced spin-orbit torques drives the application of spintronics in memory and neural networks. Given the intrinsic strong spin-orbit coupling, topological insulators (TI) with spin-momentum locking are expected to be promising candidates for generating a significant spin-orbit torque compared to the heavy metal system. To achieve high charge-to-spin conversion efficiency, it is imperative to incorporate a ferromagnetic layer with low conductivity. In this study, a high spin-torque efficiency (β<sub><i>L</i></sub> = 12.9 × 10<sup>−6</sup>mT A<sup>−1</sup>cm<sup>2</sup>) and spin Hall conductivity (<span data-altimg=\"/cms/asset/21ef69f9-2c1a-4708-b342-17fccbd6db9a/aelm1120-math-0001.png\"></span><mjx-container ctxtmenu_counter=\"13\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/aelm1120-math-0001.png\"><mjx-semantics><mjx-mrow data-semantic-children=\"5,32\" data-semantic-content=\"6\" data-semantic- data-semantic-role=\"equality\" data-semantic-speech=\"sigma Subscript upper S upper H Baseline equals 4.8 times 10 Superscript 6 Baseline StartFraction italic h over two pi Over 2 e EndFraction normal upper Omega Superscript negative 1 Baseline normal m Superscript negative 1\" data-semantic-type=\"relseq\"><mjx-msub data-semantic-children=\"0,4\" data-semantic- data-semantic-parent=\"33\" 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data-semantic-type=\"operator\"><mjx-c></mjx-c></mjx-mo><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-parent=\"4\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\"><mjx-c></mjx-c></mjx-mi></mjx-mrow></mjx-script></mjx-msub><mjx-mo data-semantic- data-semantic-operator=\"relseq,=\" data-semantic-parent=\"33\" data-semantic-role=\"equality\" data-semantic-type=\"relation\" rspace=\"5\" space=\"5\"><mjx-c></mjx-c></mjx-mo><mjx-mrow data-semantic-children=\"7,31\" data-semantic-content=\"8\" data-semantic- data-semantic-parent=\"33\" data-semantic-role=\"unknown\" data-semantic-type=\"infixop\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"32\" data-semantic-role=\"float\" data-semantic-type=\"number\"><mjx-c></mjx-c><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mn><mjx-mo data-semantic- data-semantic-operator=\"infixop,×\" data-semantic-parent=\"32\" data-semantic-role=\"unknown\" data-semantic-type=\"operator\" rspace=\"4\" space=\"4\"><mjx-c></mjx-c></mjx-mo><mjx-mrow data-semantic-annotation=\"clearspeak:unit\" data-semantic-children=\"11,17,22,27\" data-semantic-content=\"28,29,30\" data-semantic- data-semantic-parent=\"32\" data-semantic-role=\"implicit\" data-semantic-type=\"infixop\"><mjx-msup data-semantic-children=\"9,10\" data-semantic- data-semantic-parent=\"31\" data-semantic-role=\"integer\" data-semantic-type=\"superscript\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"11\" data-semantic-role=\"integer\" data-semantic-type=\"number\"><mjx-c></mjx-c><mjx-c></mjx-c></mjx-mn><mjx-script style=\"vertical-align: 0.393em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"11\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c></mjx-c></mjx-mn></mjx-script></mjx-msup><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"31\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\" style=\"margin-left: 0.056em; margin-right: 0.056em;\"><mjx-c></mjx-c></mjx-mo><mjx-mfrac data-semantic-children=\"12,16\" data-semantic- data-semantic-parent=\"31\" data-semantic-role=\"division\" data-semantic-type=\"fraction\"><mjx-frac><mjx-num><mjx-nstrut></mjx-nstrut><mjx-mi data-semantic- data-semantic-parent=\"17\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\" size=\"s\"><mjx-c></mjx-c></mjx-mi></mjx-num><mjx-dbox><mjx-dtable><mjx-line></mjx-line><mjx-row><mjx-den><mjx-dstrut></mjx-dstrut><mjx-mrow data-semantic-annotation=\"clearspeak:simple;clearspeak:unit\" data-semantic-children=\"13,14\" data-semantic-content=\"15\" data-semantic- data-semantic-parent=\"17\" data-semantic-role=\"implicit\" data-semantic-type=\"infixop\" size=\"s\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"16\" data-semantic-role=\"integer\" data-semantic-type=\"number\"><mjx-c></mjx-c></mjx-mn><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"16\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"><mjx-c></mjx-c></mjx-mo><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-parent=\"16\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\"><mjx-c></mjx-c></mjx-mi></mjx-mrow></mjx-den></mjx-row></mjx-dtable></mjx-dbox></mjx-frac></mjx-mfrac><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"31\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\" style=\"margin-left: 0.056em; margin-right: 0.056em;\"><mjx-c></mjx-c></mjx-mo><mjx-msup data-semantic-children=\"18,21\" data-semantic- data-semantic-parent=\"31\" data-semantic-role=\"greekletter\" data-semantic-type=\"superscript\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"22\" data-semantic-role=\"greekletter\" data-semantic-type=\"identifier\"><mjx-c></mjx-c></mjx-mi><mjx-script style=\"vertical-align: 0.363em;\"><mjx-mrow data-semantic-annotation=\"clearspeak:simple\" data-semantic-children=\"20\" data-semantic-content=\"19\" data-semantic- data-semantic-parent=\"22\" data-semantic-role=\"negative\" data-semantic-type=\"prefixop\" size=\"s\"><mjx-mo data-semantic- data-semantic-operator=\"prefixop,−\" data-semantic-parent=\"21\" data-semantic-role=\"subtraction\" data-semantic-type=\"operator\" rspace=\"1\"><mjx-c></mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"21\" data-semantic-role=\"integer\" data-semantic-type=\"number\"><mjx-c></mjx-c></mjx-mn></mjx-mrow></mjx-script></mjx-msup><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"31\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\" style=\"margin-left: 0.056em; margin-right: 0.056em;\"><mjx-c></mjx-c></mjx-mo><mjx-msup data-semantic-children=\"23,26\" data-semantic- data-semantic-parent=\"31\" data-semantic-role=\"latinletter\" data-semantic-type=\"superscript\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"27\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\"><mjx-c></mjx-c></mjx-mi><mjx-script style=\"vertical-align: 0.363em;\"><mjx-mrow data-semantic-annotation=\"clearspeak:simple\" data-semantic-children=\"25\" data-semantic-content=\"24\" data-semantic- data-semantic-parent=\"27\" data-semantic-role=\"negative\" data-semantic-type=\"prefixop\" size=\"s\"><mjx-mo data-semantic- data-semantic-operator=\"prefixop,−\" data-semantic-parent=\"26\" data-semantic-role=\"subtraction\" data-semantic-type=\"operator\" rspace=\"1\"><mjx-c></mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"26\" data-semantic-role=\"integer\" data-semantic-type=\"number\"><mjx-c></mjx-c></mjx-mn></mjx-mrow></mjx-script></mjx-msup></mjx-mrow></mjx-mrow></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:2199160X:media:aelm1120:aelm1120-math-0001\" display=\"inline\" location=\"graphic/aelm1120-math-0001.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow data-semantic-=\"\" data-semantic-children=\"5,32\" data-semantic-content=\"6\" data-semantic-role=\"equality\" data-semantic-speech=\"sigma Subscript upper S upper H Baseline equals 4.8 times 10 Superscript 6 Baseline StartFraction italic h over two pi Over 2 e EndFraction normal upper Omega Superscript negative 1 Baseline normal m Superscript negative 1\" data-semantic-type=\"relseq\"><msub data-semantic-=\"\" data-semantic-children=\"0,4\" data-semantic-parent=\"33\" data-semantic-role=\"greekletter\" data-semantic-type=\"subscript\"><mi data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic-parent=\"5\" data-semantic-role=\"greekletter\" data-semantic-type=\"identifier\">σ</mi><mrow data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple;clearspeak:unit\" data-semantic-children=\"1,2\" data-semantic-content=\"3\" data-semantic-parent=\"5\" data-semantic-role=\"implicit\" data-semantic-type=\"infixop\"><mi data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic-parent=\"4\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\">S</mi><mo data-semantic-=\"\" data-semantic-added=\"true\" data-semantic-operator=\"infixop,\" data-semantic-parent=\"4\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"></mo><mi data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic-parent=\"4\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\">H</mi></mrow></msub><mo data-semantic-=\"\" data-semantic-operator=\"relseq,=\" data-semantic-parent=\"33\" data-semantic-role=\"equality\" data-semantic-type=\"relation\">=</mo><mrow data-semantic-=\"\" data-semantic-children=\"7,31\" data-semantic-content=\"8\" data-semantic-parent=\"33\" data-semantic-role=\"unknown\" data-semantic-type=\"infixop\"><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"32\" data-semantic-role=\"float\" data-semantic-type=\"number\">4.8</mn><mo data-semantic-=\"\" data-semantic-operator=\"infixop,×\" data-semantic-parent=\"32\" data-semantic-role=\"unknown\" data-semantic-type=\"operator\">×</mo><mrow data-semantic-=\"\" data-semantic-annotation=\"clearspeak:unit\" data-semantic-children=\"11,17,22,27\" data-semantic-content=\"28,29,30\" data-semantic-parent=\"32\" data-semantic-role=\"implicit\" data-semantic-type=\"infixop\"><msup data-semantic-=\"\" data-semantic-children=\"9,10\" data-semantic-parent=\"31\" data-semantic-role=\"integer\" data-semantic-type=\"superscript\"><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"11\" data-semantic-role=\"integer\" data-semantic-type=\"number\">10</mn><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"11\" data-semantic-role=\"integer\" data-semantic-type=\"number\">6</mn></msup><mo data-semantic-=\"\" data-semantic-added=\"true\" data-semantic-operator=\"infixop,\" data-semantic-parent=\"31\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"></mo><mfrac data-semantic-=\"\" data-semantic-children=\"12,16\" data-semantic-parent=\"31\" data-semantic-role=\"division\" data-semantic-type=\"fraction\"><mi data-semantic-=\"\" data-semantic-parent=\"17\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\">ℏ</mi><mrow data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple;clearspeak:unit\" data-semantic-children=\"13,14\" data-semantic-content=\"15\" data-semantic-parent=\"17\" data-semantic-role=\"implicit\" data-semantic-type=\"infixop\"><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"16\" data-semantic-role=\"integer\" data-semantic-type=\"number\">2</mn><mo data-semantic-=\"\" data-semantic-added=\"true\" data-semantic-operator=\"infixop,\" data-semantic-parent=\"16\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"></mo><mi data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic-parent=\"16\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\">e</mi></mrow></mfrac><mo data-semantic-=\"\" data-semantic-added=\"true\" data-semantic-operator=\"infixop,\" data-semantic-parent=\"31\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"></mo><msup data-semantic-=\"\" data-semantic-children=\"18,21\" data-semantic-parent=\"31\" data-semantic-role=\"greekletter\" data-semantic-type=\"superscript\"><mi data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"22\" data-semantic-role=\"greekletter\" data-semantic-type=\"identifier\" mathvariant=\"normal\">Ω</mi><mrow data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-children=\"20\" data-semantic-content=\"19\" data-semantic-parent=\"22\" data-semantic-role=\"negative\" data-semantic-type=\"prefixop\"><mo data-semantic-=\"\" data-semantic-operator=\"prefixop,−\" data-semantic-parent=\"21\" data-semantic-role=\"subtraction\" data-semantic-type=\"operator\">−</mo><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"21\" data-semantic-role=\"integer\" data-semantic-type=\"number\">1</mn></mrow></msup><mo data-semantic-=\"\" data-semantic-added=\"true\" data-semantic-operator=\"infixop,\" data-semantic-parent=\"31\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"></mo><msup data-semantic-=\"\" data-semantic-children=\"23,26\" data-semantic-parent=\"31\" data-semantic-role=\"latinletter\" data-semantic-type=\"superscript\"><mi data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"27\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\" mathvariant=\"normal\">m</mi><mrow data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-children=\"25\" data-semantic-content=\"24\" data-semantic-parent=\"27\" data-semantic-role=\"negative\" data-semantic-type=\"prefixop\"><mo data-semantic-=\"\" data-semantic-operator=\"prefixop,−\" data-semantic-parent=\"26\" data-semantic-role=\"subtraction\" data-semantic-type=\"operator\">−</mo><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"26\" data-semantic-role=\"integer\" data-semantic-type=\"number\">1</mn></mrow></msup></mrow></mrow></mrow>${\\sigma _{SH}} = 4.8 \\times {10^6}\\frac{\\hbar }{{2e}}{{{\\Omega}}^{ - 1}}{{\\mathrm{m}}^{ - 1}}$</annotation></semantics></math></mjx-assistive-mml></mjx-container>) are reported as being observed at 80 K in a Cr<sub>2</sub>Te<sub>3</sub>/(Bi<sub>0.5</sub>Sb<sub>0.5</sub>)<sub>2</sub>Te<sub>3</sub> bilayer. The magnetization switching induced by spin-orbit torque in a Cr<sub>2</sub>Te<sub>3</sub>/(Bi<sub>0.5</sub>Sb<sub>0.5</sub>)<sub>2</sub>Te<sub>3</sub> bilayer is observed. It is demonstrated that the hump-like feature in the anomalous Hall effect (AHE) resistance curve can be attributed to the presence of two magnetic phases in compressively strained chromium telluride grown on a <i>c</i>-Al<sub>2</sub>O<sub>3</sub> substrate using molecular beam epitaxy (MBE). The work holds the promise of propelling efficiency advancements in spintronic applications that leverage the unique properties of topological insulators.","PeriodicalId":110,"journal":{"name":"Advanced Electronic Materials","volume":"16 1","pages":""},"PeriodicalIF":5.3000,"publicationDate":"2025-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Electronic Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/aelm.202400820","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Energy-efficient magnetization switching by current-induced spin-orbit torques drives the application of spintronics in memory and neural networks. Given the intrinsic strong spin-orbit coupling, topological insulators (TI) with spin-momentum locking are expected to be promising candidates for generating a significant spin-orbit torque compared to the heavy metal system. To achieve high charge-to-spin conversion efficiency, it is imperative to incorporate a ferromagnetic layer with low conductivity. In this study, a high spin-torque efficiency (βL = 12.9 × 10−6mT A−1cm2) and spin Hall conductivity () are reported as being observed at 80 K in a Cr2Te3/(Bi0.5Sb0.5)2Te3 bilayer. The magnetization switching induced by spin-orbit torque in a Cr2Te3/(Bi0.5Sb0.5)2Te3 bilayer is observed. It is demonstrated that the hump-like feature in the anomalous Hall effect (AHE) resistance curve can be attributed to the presence of two magnetic phases in compressively strained chromium telluride grown on a c-Al2O3 substrate using molecular beam epitaxy (MBE). The work holds the promise of propelling efficiency advancements in spintronic applications that leverage the unique properties of topological insulators.
期刊介绍:
Advanced Electronic Materials is an interdisciplinary forum for peer-reviewed, high-quality, high-impact research in the fields of materials science, physics, and engineering of electronic and magnetic materials. It includes research on physics and physical properties of electronic and magnetic materials, spintronics, electronics, device physics and engineering, micro- and nano-electromechanical systems, and organic electronics, in addition to fundamental research.