The Golden Age of Thermally Activated Delayed Fluorescence Materials: Design and Exploitation

IF 51.4 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Chemical Reviews Pub Date : 2024-12-12 DOI:10.1021/acs.chemrev.3c00755

John Marques Dos Santos, David Hall, Biju Basumatary, Megan Bryden, Dongyang Chen, Praveen Choudhary, Thomas Comerford, Ettore Crovini, Andrew Danos, Joydip De, Stefan Diesing, Mahni Fatahi, Máire Griffin, Abhishek Kumar Gupta, Hassan Hafeez, Lea Hämmerling, Emily Hanover, Janine Haug, Tabea Heil, Durai Karthik, Shiv Kumar, Oliver Lee, Haoyang Li, Fabien Lucas, Campbell Frank Ross Mackenzie, Aminata Mariko, Tomas Matulaitis, Francis Millward, Yoann Olivier, Quan Qi, Ifor D. W. Samuel, Nidhi Sharma, Changfeng Si, Leander Spierling, Pagidi Sudhakar, Dianming Sun, Eglė Tankelevičiu̅tė, Michele Duarte Tonet, Jingxiang Wang, Tao Wang, Sen Wu, Yan Xu, Le Zhang, Eli Zysman-Colman

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Abstract

Since the seminal report by Adachi and co-workers in 2012, there has been a veritable explosion of interest in the design of thermally activated delayed fluorescence (TADF) compounds, particularly as emitters for organic light-emitting diodes (OLEDs). With rapid advancements and innovation in materials design, the efficiencies of TADF OLEDs for each of the primary color points as well as for white devices now rival those of state-of-the-art phosphorescent emitters. Beyond electroluminescent devices, TADF compounds have also found increasing utility and applications in numerous related fields, from photocatalysis, to sensing, to imaging and beyond. Following from our previous review in 2017 ( Adv. Mater. 2017, 1605444), we here comprehensively document subsequent advances made in TADF materials design and their uses from 2017–2022. Correlations highlighted between structure and properties as well as detailed comparisons and analyses should assist future TADF materials development. The necessarily broadened breadth and scope of this review attests to the bustling activity in this field. We note that the rapidly expanding and accelerating research activity in TADF material development is indicative of a field that has reached adolescence, with an exciting maturity still yet to come.

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热活化延迟荧光材料的黄金时代：设计与开发

自2012年安达立及其同事发表开创性报告以来，人们对热激活延迟荧光（TADF）化合物的设计，特别是作为有机发光二极管（oled）的发射器，产生了真正的兴趣。随着材料设计的快速发展和创新，TADF oled在每个原色点以及白色器件上的效率现在可以与最先进的磷光发射器相媲美。除了电致发光器件之外，TADF化合物也在许多相关领域中发现了越来越多的用途和应用，从光催化，到传感，到成像等等。根据我们在2017年的上一次审查（Adv. Mater. 2017,1605444），我们在这里全面记录了2017 - 2022年期间TADF材料设计及其使用的后续进展。强调结构和性能之间的相关性以及详细的比较和分析将有助于未来TADF材料的开发。这一审查的广度和范围必然扩大，这证明了这一领域的繁忙活动。我们注意到，在TADF材料开发方面迅速扩大和加速的研究活动表明，这一领域已进入青春期，令人兴奋的成熟尚未到来。

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来源期刊

Chemical Reviews 化学-化学综合

CiteScore

106.00

自引率

1.10%

发文量

278

审稿时长

4.3 months

期刊介绍： Chemical Reviews is a highly regarded and highest-ranked journal covering the general topic of chemistry. Its mission is to provide comprehensive, authoritative, critical, and readable reviews of important recent research in organic, inorganic, physical, analytical, theoretical, and biological chemistry. Since 1985, Chemical Reviews has also published periodic thematic issues that focus on a single theme or direction of emerging research.