The Golden Age of Thermally Activated Delayed Fluorescence Materials: Design and Exploitation

IF 51.4 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Chemical Reviews Pub Date : 2024-12-12 DOI:10.1021/acs.chemrev.3c00755

John Marques Dos Santos, David Hall, Biju Basumatary, Megan Bryden, Dongyang Chen, Praveen Choudhary, Thomas Comerford, Ettore Crovini, Andrew Danos, Joydip De, Stefan Diesing, Mahni Fatahi, Máire Griffin, Abhishek Kumar Gupta, Hassan Hafeez, Lea Hämmerling, Emily Hanover, Janine Haug, Tabea Heil, Durai Karthik, Shiv Kumar, Oliver Lee, Haoyang Li, Fabien Lucas, Campbell Frank Ross Mackenzie, Aminata Mariko, Tomas Matulaitis, Francis Millward, Yoann Olivier, Quan Qi, Ifor D. W. Samuel, Nidhi Sharma, Changfeng Si, Leander Spierling, Pagidi Sudhakar, Dianming Sun, Eglė Tankelevičiu̅tė, Michele Duarte Tonet, Jingxiang Wang, Tao Wang, Sen Wu, Yan Xu, Le Zhang, Eli Zysman-Colman

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Abstract

Since the seminal report by Adachi and co-workers in 2012, there has been a veritable explosion of interest in the design of thermally activated delayed fluorescence (TADF) compounds, particularly as emitters for organic light-emitting diodes (OLEDs). With rapid advancements and innovation in materials design, the efficiencies of TADF OLEDs for each of the primary color points as well as for white devices now rival those of state-of-the-art phosphorescent emitters. Beyond electroluminescent devices, TADF compounds have also found increasing utility and applications in numerous related fields, from photocatalysis, to sensing, to imaging and beyond. Following from our previous review in 2017 ( Adv. Mater. 2017, 1605444), we here comprehensively document subsequent advances made in TADF materials design and their uses from 2017–2022. Correlations highlighted between structure and properties as well as detailed comparisons and analyses should assist future TADF materials development. The necessarily broadened breadth and scope of this review attests to the bustling activity in this field. We note that the rapidly expanding and accelerating research activity in TADF material development is indicative of a field that has reached adolescence, with an exciting maturity still yet to come.

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来源期刊

Chemical Reviews 化学-化学综合

CiteScore

106.00

自引率

1.10%

发文量

278

审稿时长

4.3 months

期刊介绍： Chemical Reviews is a highly regarded and highest-ranked journal covering the general topic of chemistry. Its mission is to provide comprehensive, authoritative, critical, and readable reviews of important recent research in organic, inorganic, physical, analytical, theoretical, and biological chemistry. Since 1985, Chemical Reviews has also published periodic thematic issues that focus on a single theme or direction of emerging research.