Electrode/Electrolyte Optimization-Induced Double-Layered Architecture for High-Performance Aqueous Zinc-(Dual) Halogen Batteries

IF 26.6 1区材料科学 Q1 Engineering

Nano-Micro Letters Pub Date : 2024-11-07 DOI:10.1007/s40820-024-01551-w

Chengwang Zhou, Zhezheng Ding, Shengzhe Ying, Hao Jiang, Yan Wang, Timing Fang, You Zhang, Bing Sun, Xiao Tang, Xiaomin Liu

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Abstract

Highlights

A double-layered protective film based on zinc-based coordination compound and ZnF₂-rich solid electrolyte interphase layer has been successfully fabricated on the zinc metal anode via electrode/electrolyte synergistic optimization.
The double-layered architecture can effectively modulate Zn²⁺ flux and suppress the zinc dendrite growth, thus facilitating the uniform zinc deposition.
The as-developed zinc-(dual) halogen batteries based on double-layered protective film can present high areal capacity and satisfactory cycling stability.

Abstract Image

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电极/电解质优化--高性能水性锌-（双）卤素电池的双层结构

通过电极/电解质协同优化，在锌金属阳极上成功制备了基于锌基配位化合物和富含 ZnF2 的固体电解质相间层的双层保护膜。双层结构可有效调节 Zn2+ 通量并抑制锌枝晶的生长，从而促进锌的均匀沉积。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Nano-Micro Letters NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY

CiteScore

32.60

自引率

4.90%

发文量

981

审稿时长

1.1 months

期刊介绍： Nano-Micro Letters is a peer-reviewed, international, interdisciplinary, and open-access journal published under the SpringerOpen brand. Nano-Micro Letters focuses on the science, experiments, engineering, technologies, and applications of nano- or microscale structures and systems in various fields such as physics, chemistry, biology, material science, and pharmacy.It also explores the expanding interfaces between these fields. Nano-Micro Letters particularly emphasizes the bottom-up approach in the length scale from nano to micro. This approach is crucial for achieving industrial applications in nanotechnology, as it involves the assembly, modification, and control of nanostructures on a microscale.