Polyacrylamide-modified nitrogen-doped carbon as a high-performance electrode for electrosorption of uranium from wastewater

IF 1.5 3区 化学 Q3 CHEMISTRY, ANALYTICAL
Meng Cao, Liman Chen, Jiaqi Chen, Yunyang Gui, Peng Liu, Yongde Yan, Yun Xue
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Abstract

As an energy-saving and facile technology, electrosorption technology has good potential in the process of separation of uranium from aqueous solution. In this study, sucrose and urea were used to prepare nitrogen-doped carbon by one-step carbonization, and polyacrylamide modified nitrogen doped carbon (PAM/NC) was obtained by modification. The electrosorption test results indicated that PAM/NC-2 had the best properties and the maximum electrosorption capacity was 619.5 mg g−1. The performance loss was less than 20% after 5 adsorption–desorption cycles. Overall, this material had a potential application in U(VI) pollution remediation, meeting the need for sustainable development of nuclear energy.

Abstract Image

聚丙烯酰胺改性掺氮碳作为电吸附废水中铀的高性能电极
电吸附技术作为一种节能、简便的技术,在从水溶液中分离铀的过程中具有良好的潜力。本研究采用蔗糖和尿素一步碳化法制备掺氮炭,通过改性得到聚丙烯酰胺改性掺氮炭(PAM/NC)。电吸附测试结果表明,PAM/NC-2 的性能最好,最大电吸附容量为 619.5 mg g-1。经过 5 次吸附-解吸循环后,性能损失小于 20%。总体而言,这种材料在六(U)铀污染修复方面具有潜在的应用价值,满足了核能可持续发展的需要。
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来源期刊
CiteScore
2.80
自引率
18.80%
发文量
504
审稿时长
2.2 months
期刊介绍: An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.
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