Electrocatalytic organic transformation reactions in green chemistry: Exploring nanocrystals and single atom catalysts

IF 9.5 2区材料科学 Q1 CHEMISTRY, PHYSICAL

Nano Research Pub Date : 2024-08-09 DOI:10.1007/s12274-024-6887-8

Ziwei Deng, Yuexin Guo, Zhiyi Sun, Jie Lin, Huazhang Zhai, Wenxing Chen

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Abstract

Organic synthesis chemistry plays a crucial role in supporting social sustainable development and finds widespread applications across various fields. Electrocatalysis, with its benefits of high efficiency, mild reaction conditions, controllability, and environmental friendliness, stands out as one of the most effective strategies for driving the transformation of organic substrates. In recent years, nanocrystals (NCs) and single atom catalysts (SACs) have garnered significant attention in the realm of electrocatalytic organic transformation. This article presents a comprehensive overview of the applications of NCs and SACs in electrocatalytic organic transformation. It delves into advanced catalysts for electrocatalysis of representative substrates, covering both anodic oxidation and cathodic reduction aspects, and addresses their synthesis, characterization, catalytic mechanism, and performance. The ultimate goal of this review is to serve as a valuable reference and a source of inspiration for further exploration into the development of more effective catalysts for electrocatalytic organic transformation.

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绿色化学中的电催化有机转化反应：探索纳米晶体和单原子催化剂

有机合成化学在支持社会可持续发展方面发挥着至关重要的作用，并在各个领域得到广泛应用。电催化具有效率高、反应条件温和、可控性强、环境友好等优点，是推动有机基质转化的最有效策略之一。近年来，纳米晶体（NCs）和单原子催化剂（SACs）在电催化有机转化领域备受关注。本文全面概述了 NC 和 SAC 在电催化有机转化中的应用。文章深入探讨了用于代表性基质电催化的先进催化剂，涵盖阳极氧化和阴极还原两个方面，并讨论了它们的合成、表征、催化机理和性能。本综述的最终目的是为进一步探索开发更有效的电催化有机转化催化剂提供有价值的参考和灵感来源。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Nano Research 化学-材料科学：综合

CiteScore

14.30

自引率

11.10%

发文量

2574

审稿时长

1.7 months

期刊介绍： Nano Research is a peer-reviewed, international and interdisciplinary research journal that focuses on all aspects of nanoscience and nanotechnology. It solicits submissions in various topical areas, from basic aspects of nanoscale materials to practical applications. The journal publishes articles on synthesis, characterization, and manipulation of nanomaterials; nanoscale physics, electrical transport, and quantum physics; scanning probe microscopy and spectroscopy; nanofluidics; nanosensors; nanoelectronics and molecular electronics; nano-optics, nano-optoelectronics, and nano-photonics; nanomagnetics; nanobiotechnology and nanomedicine; and nanoscale modeling and simulations. Nano Research offers readers a combination of authoritative and comprehensive Reviews, original cutting-edge research in Communication and Full Paper formats. The journal also prioritizes rapid review to ensure prompt publication.