{"title":"Multifunctional biopolymer poly (lactic acid)-based triboelectric nanogenerator via controlled construction of secondary electron path","authors":"Tairong Kuang , Jingbing Zhang , Guang-Ming Huang , Tong Liu , Zhao-Xia Huang","doi":"10.1016/j.nanoen.2024.109877","DOIUrl":null,"url":null,"abstract":"<div><p>Seeking sustainable energy solutions for bioelectronic devices, high-performance, multifunctional biopolymer-based triboelectric nanogenerators (TENGs) are proving to be essential for biomedical applications. This study presents an innovative fabrication method for establishing secondary electron transport paths, resulting in biopolymer-based nanocomposites (poly (lactic acid) (PLA)/carbon nanotube (CNT)@expanded graphite (EG)) with inherent electron pathways. By integrating conductive biopolymer nanocomposites with polytetrafluoroethylene (PTFE) films, we developed a contact-separation mode TENG (CS-TENG) that demonstrates outstanding energy-harvesting efficiency. The CS-TENG displays an impressive charge density of 280 μC/m<sup>2</sup>, accompanied by an open circuit voltage (V<sub>oc</sub>) of 100.5 V and short circuit current density (I<sub>sc</sub>) values of 47.25 mA/m<sup>2</sup>. Moreover, the essential conductive network guarantees the CS-TENG’s stability across different humidity levels and serves as a moisture barrier. In addition to energy harvesting, the fabricated biopolymer nanocomposite films exhibit effective electromagnetic interference (EMI) shielding and Joule heating capabilities, rendering the CS-TENG suitable for use in diverse application scenarios. Our results emphasize the crucial role of conductive network architecture in creating high-performance biopolymer PLA-based TENGs. The innovative fabrication method and our CS-TENG's capabilities reveal the significant potential of biopolymer-based composites to transform energy harvesting, thermal management, and EMI shielding in bioelectronics.</p></div>","PeriodicalId":394,"journal":{"name":"Nano Energy","volume":null,"pages":null},"PeriodicalIF":16.8000,"publicationDate":"2024-06-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Energy","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2211285524006256","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Seeking sustainable energy solutions for bioelectronic devices, high-performance, multifunctional biopolymer-based triboelectric nanogenerators (TENGs) are proving to be essential for biomedical applications. This study presents an innovative fabrication method for establishing secondary electron transport paths, resulting in biopolymer-based nanocomposites (poly (lactic acid) (PLA)/carbon nanotube (CNT)@expanded graphite (EG)) with inherent electron pathways. By integrating conductive biopolymer nanocomposites with polytetrafluoroethylene (PTFE) films, we developed a contact-separation mode TENG (CS-TENG) that demonstrates outstanding energy-harvesting efficiency. The CS-TENG displays an impressive charge density of 280 μC/m2, accompanied by an open circuit voltage (Voc) of 100.5 V and short circuit current density (Isc) values of 47.25 mA/m2. Moreover, the essential conductive network guarantees the CS-TENG’s stability across different humidity levels and serves as a moisture barrier. In addition to energy harvesting, the fabricated biopolymer nanocomposite films exhibit effective electromagnetic interference (EMI) shielding and Joule heating capabilities, rendering the CS-TENG suitable for use in diverse application scenarios. Our results emphasize the crucial role of conductive network architecture in creating high-performance biopolymer PLA-based TENGs. The innovative fabrication method and our CS-TENG's capabilities reveal the significant potential of biopolymer-based composites to transform energy harvesting, thermal management, and EMI shielding in bioelectronics.
期刊介绍：
Nano Energy is a multidisciplinary, rapid-publication forum of original peer-reviewed contributions on the science and engineering of nanomaterials and nanodevices used in all forms of energy harvesting, conversion, storage, utilization and policy. Through its mixture of articles, reviews, communications, research news, and information on key developments, Nano Energy provides a comprehensive coverage of this exciting and dynamic field which joins nanoscience and nanotechnology with energy science. The journal is relevant to all those who are interested in nanomaterials solutions to the energy problem.
Nano Energy publishes original experimental and theoretical research on all aspects of energy-related research which utilizes nanomaterials and nanotechnology. Manuscripts of four types are considered: review articles which inform readers of the latest research and advances in energy science; rapid communications which feature exciting research breakthroughs in the field; full-length articles which report comprehensive research developments; and news and opinions which comment on topical issues or express views on the developments in related fields.
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