Modeling Multicomponent Fluid Flow in Deforming and Reacting Porous Rock

IF 1 4区 地球科学 Q3 GEOCHEMISTRY & GEOPHYSICS
L. Khakimova, Yu. Podladchikov
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Abstract

We propose a coupled hydro-mechanical-chemical model and its 1D numerical implementation. We demonstrate its application to the model filtration of a multicomponent fluid in deforming and reacting host rocks, considering changes in the densities, phase proportions, and the chemical compositions of the coexisting phases. The presented 1D numerical implementation is illustrated by the example of soapstone formation from serpentinite during the filtration of Н2О−CО2 fluid with a low CО2 concentration coupled with the viscous deformation of the mineral matrix, considering the MgO−SiO2−Н2О−CО2 system. The numerical results show the propagation of a porosity wave by means of a viscous (de)compaction mechanism accompanied by the formation of an elongated zone with higher filtration properties. After the formation of such a channel, the formation and propagation of the reaction fronts occur and are associated with the transformation of the mineral composition of the original rock. During H2O−CO2 fluid filtration, starting with 1 wt % dissolved CO2, carbonization of hydrated serpentinite starts, specifically antigorite transforms to magnesite and talc.

Abstract Image

Abstract Image

多孔岩石变形和反应过程中的多组分流体流动建模
摘要 我们提出了一种水文-机械-化学耦合模型及其一维数值实施方法。考虑到共存相的密度、相比例和化学成分的变化,我们展示了该模型在多组分流体在变形和反应母岩中过滤的应用。考虑到 MgO-SiO2-Н2О-CО2 体系,以蛇纹岩形成皂石为例,说明了在低 CО2 浓度的 Н2О-CО2 流体过滤过程中,以及矿物基质的粘性变形过程中,所提出的一维数值实现方法。数值结果表明,孔隙波是通过粘性(去)压实机制传播的,并伴随着具有更高过滤特性的拉长区域的形成。在这种通道形成后,反应锋的形成和传播与原岩矿物成分的转变有关。在 H2O-CO2 流体过滤过程中,从溶解度为 1 wt % 的 CO2 开始,水合蛇绿岩开始碳化,特别是锑橄榄石转变为菱镁矿和滑石。
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来源期刊
Petrology
Petrology 地学-地球科学综合
CiteScore
2.40
自引率
20.00%
发文量
27
审稿时长
>12 weeks
期刊介绍: Petrology is a journal of magmatic, metamorphic, and experimental petrology, mineralogy, and geochemistry. The journal offers comprehensive information on all multidisciplinary aspects of theoretical, experimental, and applied petrology. By giving special consideration to studies on the petrography of different regions of the former Soviet Union, Petrology provides readers with a unique opportunity to refine their understanding of the geology of the vast territory of the Eurasian continent. The journal welcomes manuscripts from all countries in the English or Russian language.
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