Study on the influence of different thermal coals on the mixed-burning characteristics of ventilation air methane and pulverized coal

IF 2.7 4区 环境科学与生态学 Q3 ENERGY & FUELS
Chaoyu Hao, Yufei Liu, Yankun Chen, Yachao Zhang, Cunbao Deng
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Abstract

To effectively utilize ventilation air methane (VAM), it is proposed to pass it into the boiler of the coal-fired power plant for mixed combustion. However, the different types of thermal coal utilized present distinct characteristics when mixed with VAM. In this paper, lignite, bituminous coal, and anthracite are selected to study the CH4 conversion rate, system ignition temperature, and NO emission characteristics of the VAM-pulverized coal coupled system on a fluidized bed experimental platform. The experimental results show that the ignition temperatures of VAM are 748, 736, and 732 °C when the CH4 concentration is 0.25, 0.5, and 0.75%. After the addition of thermal coal, the ignition temperature decreased significantly. When the CH4 concentration is 0.25%, the ignition temperature of the lignite-VAM system is the lowest, which is 450 °C. Anthracite has the strongest catalytic effect on CH4 combustion. When the heating rate is 5 °C /min, the reaction rate of CH4 is the fastest in the anthracite-VAM coupled system. Under laboratory conditions, the peak NO concentration in the coal-VAM coupled system was lignite > bituminous coal > anthracite at different CH4 concentrations, and the CH4 in VAM had a reducing action on the NO generated during mixed combustion, with a stronger reducing effect observed as the CH4 concentration increased. The results of this study can lay the foundation for the industrial application of the mixed combustion of VAM and thermal coal, and be of great significance for solving the practical problems caused by the change of boiler coal types. © 2024 Society of Chemical Industry and John Wiley & Sons, Ltd.

不同热煤对通气甲烷和煤粉混合燃烧特性的影响研究
为有效利用通风甲烷(VAM),建议将其送入燃煤发电厂的锅炉进行混合燃烧。然而,不同类型的动力煤与 VAM 混合后会呈现出不同的特性。本文选择了褐煤、烟煤和无烟煤,在流化床实验平台上研究 VAM 与粉煤耦合系统的 CH4 转化率、系统着火温度和 NO 排放特性。实验结果表明,当 CH4 浓度为 0.25%、0.5% 和 0.75%时,VAM 的着火温度分别为 748、736 和 732 ℃。加入动力煤后,着火温度明显降低。当 CH4 浓度为 0.25% 时,褐煤-VAM 系统的着火温度最低,为 450 ℃。无烟煤对 CH4 燃烧的催化作用最强。当升温速率为 5 °C /min 时,无烟煤-VAM 耦合系统中 CH4 的反应速率最快。在实验室条件下,不同CH4浓度下,煤-VAM耦合体系中的NO浓度峰值分别为褐煤、烟煤和无烟煤,VAM中的CH4对混合燃烧过程中产生的NO有还原作用,随着CH4浓度的增加,还原作用更强。该研究结果可为 VAM 与动力煤混合燃烧的工业应用奠定基础,对解决锅炉煤种变化带来的实际问题具有重要意义。© 2024 化学工业协会和约翰-威利-桑普森有限公司版权所有。
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来源期刊
Greenhouse Gases: Science and Technology
Greenhouse Gases: Science and Technology ENERGY & FUELS-ENGINEERING, ENVIRONMENTAL
CiteScore
4.90
自引率
4.50%
发文量
55
审稿时长
3 months
期刊介绍: Greenhouse Gases: Science and Technology is a new online-only scientific journal dedicated to the management of greenhouse gases. The journal will focus on methods for carbon capture and storage (CCS), as well as utilization of carbon dioxide (CO2) as a feedstock for fuels and chemicals. GHG will also provide insight into strategies to mitigate emissions of other greenhouse gases. Significant advances will be explored in critical reviews, commentary articles and short communications of broad interest. In addition, the journal will offer analyses of relevant economic and political issues, industry developments and case studies. Greenhouse Gases: Science and Technology is an exciting new online-only journal published as a co-operative venture of the SCI (Society of Chemical Industry) and John Wiley & Sons, Ltd
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