Inducing torque on molecular magnets via Laguerre Gaussian beams

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Gang Lei, Shanzhi Li
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引用次数: 0

Abstract

This theoretical study delves into the induction of torque by light beams carrying orbital angular momentum on single-molecule magnets (SMMs). The investigation explores the impact of decay rates, detunings, and control field intensities on the generation of light-induced torque and the resulting current flow in a ring formation. The results highlight the crucial role of the control field, showcasing its efficacy as a tool to manipulate and amplify torque at different frequencies. Detuning is identified as a critical parameter influencing the shift, slope, and emergence of multiple peaks in the torque profile. The interplay between detuning, control field intensity, and decay rates introduces a control mechanism for fine-tuning torque at distinct probe frequencies. These findings underscore the potential applications of the control field and detuning as robust tools for tailored manipulation of torque in SMMs, paving the way for advancements in controlled current flow dynamics with ring structures.
通过拉盖尔高斯束在分子磁体上诱导扭矩
这项理论研究深入探讨了携带轨道角动量的光束在单分子磁体(SMMs)上感应扭矩的问题。研究探讨了衰减率、失谐和控制场强度对光诱导力矩的产生以及由此产生的环形电流的影响。研究结果强调了控制场的关键作用,展示了其作为在不同频率下操纵和放大扭矩的工具的功效。解谐被认为是影响扭矩曲线中多个峰值的移动、斜率和出现的关键参数。解谐、控制场强度和衰减率之间的相互作用引入了一种控制机制,用于微调不同探针频率下的扭矩。这些发现强调了控制场和解谐作为定制操纵 SMM 扭矩的强大工具的潜在应用,为环形结构的受控电流动力学的进步铺平了道路。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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