Design and analysis of a highly efficient 2D/3D bilayer-based perovskite solar cell

IF 2.2 4区工程技术 Q3 ENGINEERING, ELECTRICAL & ELECTRONIC

Journal of Computational Electronics Pub Date : 2024-03-26 DOI:10.1007/s10825-024-02152-x

M. Najafi, A. Kiani–Sarkaleh, A. Ghadimi, S. A. Sedigh Ziabari, Ali Abdolahzadeh Ziabari

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Abstract

Despite significant development of perovskite solar cells (PSCs) in the last few years, several issues need to be addressed for commercialization. The fabrication of a 2-dimensional/3-dimensional (2D/3D) perovskite layer as the light absorbing layer has recently come up as one of the most efficient methods to overcome this barrier without compromising the physical functionality of the device. Additionally, the inverted p–i–n configuration of2D/3D bilayer PSCs has caught lots of attention in the recent years owing to low-cost, low-temperature growth process and inhibited hysteresis properties. In this study, we introduce an inverted 2D/3D bilayer PSC with a novel configuration of FTO/NiO_x/BA₂MA₃Pb₄I₁₃/MAPbI₃/C60/Au and computationally study the parameters that affect the performance of the modeled device. Considerable power conversion efficiency (PCE) of 28.24% was achieved after optimizing the performance.

Abstract Image

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设计和分析高效的基于二维/三维双层的过氧化物太阳能电池

尽管过去几年中包晶石太阳能电池（PSCs）取得了长足的发展，但要实现商业化还需要解决几个问题。最近，制造二维/三维（2D/3D）包晶石层作为光吸收层已成为克服这一障碍的最有效方法之一，而且不会影响设备的物理功能。此外，由于低成本、低温生长工艺和抑制滞后特性，2D/3D 双层 PSCs 的倒 pi-n 构型近年来引起了广泛关注。在本研究中，我们介绍了一种具有 FTO/NiOx/BA2MA3Pb4I13/MAPbI3/C60/Au 新型配置的倒置 2D/3D 双层 PSC，并对影响模型器件性能的参数进行了计算研究。优化性能后，功率转换效率 (PCE) 达到了 28.24%。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Journal of Computational Electronics ENGINEERING, ELECTRICAL & ELECTRONIC-PHYSICS, APPLIED

CiteScore

4.50

自引率

4.80%

发文量

142

审稿时长

>12 weeks

期刊介绍： he Journal of Computational Electronics brings together research on all aspects of modeling and simulation of modern electronics. This includes optical, electronic, mechanical, and quantum mechanical aspects, as well as research on the underlying mathematical algorithms and computational details. The related areas of energy conversion/storage and of molecular and biological systems, in which the thrust is on the charge transport, electronic, mechanical, and optical properties, are also covered. In particular, we encourage manuscripts dealing with device simulation; with optical and optoelectronic systems and photonics; with energy storage (e.g. batteries, fuel cells) and harvesting (e.g. photovoltaic), with simulation of circuits, VLSI layout, logic and architecture (based on, for example, CMOS devices, quantum-cellular automata, QBITs, or single-electron transistors); with electromagnetic simulations (such as microwave electronics and components); or with molecular and biological systems. However, in all these cases, the submitted manuscripts should explicitly address the electronic properties of the relevant systems, materials, or devices and/or present novel contributions to the physical models, computational strategies, or numerical algorithms.