Gas cleaning with semi-wet type plasma reactor

A. Chakrabarti, A. Mizuno, K. Shimizu, T. Matsuoka, S. Furuta
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引用次数: 39

Abstract

An experimental study on the removal of NH/sub 3/, NO, and NO/sub x/ in concentrations of 10-40 ppm in air has been carried out using plasma chemical reaction in a streamer corona discharge. The results of the performance of dry-type and semi-wet-type reactors are compared. The effect of different types of applied voltages such as rectangular pulse, 60 Hz sinusoidal, and 18 kHz alternating voltages is investigated. During NO removal, O/sub 3/ and NO/sub 2/ are produced. NO/sub 2/ can, partially, be removed with higher power input into the discharge. Another undesirable pollutant, namely N/sub 2/O, is also produced, especially in the case of dry reactors having long residence time ( approximately 2.4 s). N/sub 2/O production decreases, essentially, to zero at 0.6 s residence time when using a semiwet reactor. In general, higher removal efficiency has been obtained with pulse voltage in a wet reactor. NH/sub 3/ in air appears to produce ozone and ammonium nitrate in a discharge. The performance of semiwet reactors with regard to the removal of submicron dust particles has also been investigated and very high removal efficiency ( approximately 93% at 0.6 s residence time) has been obtained.<>
半湿式等离子体反应器气体清洗
采用流光电晕放电等离子体化学反应对空气中10 ~ 40ppm浓度的NH/sub - 3/、NO和NO/sub - x/进行了去除实验研究。对干式和半湿式反应器的性能进行了比较。研究了矩形脉冲、60hz正弦波和18khz交流电压等不同外加电压的影响。在去除NO的过程中,会产生O/sub 3/和NO/sub 2/。通过在放电中输入更高的功率,可以部分去除NO/sub 2/。另一种不希望的污染物,即N/sub - 2/O,也会产生,特别是在具有长停留时间(约2.4 s)的干式反应器的情况下。当使用半湿式反应器时,N/sub - 2/O的产生基本上在0.6 s的停留时间降至零。一般来说,在湿式反应器中使用脉冲电压可以获得较高的去除效率。在一次排放中,空气中的NH/sub /似乎会产生臭氧和硝酸铵。半湿反应器在去除亚微米粉尘方面的性能也进行了研究,并获得了非常高的去除效率(在0.6 s的停留时间内约为93%)。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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